Resonant ultrasound spectroscopy of transition metal tetrachalcogenides

During this master's thesis, the set-up of resonant ultrasound spectroscopy (RUS) technique was developed at the Universidad de los Andes and a temperature-dependent experiment was carried out.

Autores:: Cruz Castiblanco, Juan Pablo Nicolás

Tipo de recurso:: Trabajo de grado de pregrado

Fecha de publicación:: 2023

Institución:: Universidad de los Andes

Repositorio:: Séneca: repositorio Uniandes

Idioma:: spa

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repository_id_str
dc.title.eng.fl_str_mv	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
dc.title.alternative.spa.fl_str_mv	Espectroscopía de resonancia ultrasónica de calcogenuros de metales de transición
title	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
spellingShingle	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides Charge density wave NbTe4 TaTe4 Phase transitions Resonant ultrasound spectroscopy Thermal hysteresis Onda de densidad de carga NbTe4 TaTe4 Transisiones de fase Espectroscopía de resonancia ultrasónica Histéresis térmica Física
title_short	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
title_full	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
title_fullStr	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
title_full_unstemmed	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
title_sort	Resonant ultrasound spectroscopy of transition metal tetrachalcogenides
dc.creator.fl_str_mv	Cruz Castiblanco, Juan Pablo Nicolás
dc.contributor.advisor.none.fl_str_mv	Giraldo Gallo, Paula Liliana
dc.contributor.author.none.fl_str_mv	Cruz Castiblanco, Juan Pablo Nicolás
dc.contributor.jury.none.fl_str_mv	Rincón, Julián Roa, Jairo
dc.contributor.researchgroup.none.fl_str_mv	Facultad de Ciencias
dc.subject.keyword.eng.fl_str_mv	Charge density wave
topic	Charge density wave NbTe4 TaTe4 Phase transitions Resonant ultrasound spectroscopy Thermal hysteresis Onda de densidad de carga NbTe4 TaTe4 Transisiones de fase Espectroscopía de resonancia ultrasónica Histéresis térmica Física
dc.subject.keyword.none.fl_str_mv	NbTe4 TaTe4 Phase transitions Resonant ultrasound spectroscopy Thermal hysteresis Onda de densidad de carga NbTe4 TaTe4 Transisiones de fase Espectroscopía de resonancia ultrasónica Histéresis térmica
dc.subject.themes.spa.fl_str_mv	Física
description	During this master's thesis, the set-up of resonant ultrasound spectroscopy (RUS) technique was developed at the Universidad de los Andes and a temperature-dependent experiment was carried out.
publishDate	2023
dc.date.issued.none.fl_str_mv	2023-12-12
dc.date.accessioned.none.fl_str_mv	2024-01-31T20:12:44Z
dc.date.accepted.none.fl_str_mv	2024-01-30
dc.date.available.none.fl_str_mv	2025-02-19
dc.type.none.fl_str_mv	Trabajo de grado - Maestría
dc.type.driver.none.fl_str_mv	info:eu-repo/semantics/masterThesis
dc.type.version.none.fl_str_mv	info:eu-repo/semantics/acceptedVersion
dc.type.coar.none.fl_str_mv	http://purl.org/coar/resource_type/c_7a1f
dc.type.content.none.fl_str_mv	Text
dc.type.redcol.none.fl_str_mv	http://purl.org/redcol/resource_type/TP
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dc.identifier.uri.none.fl_str_mv	https://hdl.handle.net/1992/73704
dc.identifier.instname.none.fl_str_mv	instname:Universidad de los Andes
dc.identifier.reponame.none.fl_str_mv	reponame:Repositorio Institucional Séneca
dc.identifier.repourl.none.fl_str_mv	repourl:https://repositorio.uniandes.edu.co/
url	https://hdl.handle.net/1992/73704
identifier_str_mv	instname:Universidad de los Andes reponame:Repositorio Institucional Séneca repourl:https://repositorio.uniandes.edu.co/
dc.language.iso.none.fl_str_mv	spa
language	spa
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Metals 2017, Vol. 7, Page 215, 7:215, 6 2017. R. I. Zainullina, N. G. Bebenin, V. V. Mashkautsan, V. V. Ustinov, and Ya M. Mukovskii. Giant thermal hysteresis in lanthanum manganites. Journal of Magnetism and Magnetic Materials, 300:e137–e139, 5 2006. Marco Scalerandi, Valentina Agostini, Pier Paolo Delsanto, Koen Van Den Abeele, and Paul A. Johnson. Local interaction simulation approach to modelling nonclassical, nonlinear elastic behavior in solids. The Journal of the Acoustical Society of America, 113:3049–3059, 6 2003. James A. TenCate, Eric Smith, and Robert A. Guyer. Universal slow dynamics in granular solids. Physical Review Letters, 85:1020, 7 2000. James A. TenCate. Slow dynamics of earth materials: An experimental overview. Pure and Applied Geophysics, 168:2211–2219, 12 2011. Yening Wang, Linhai Sun, Jin Wu, and Min Gu. Thermal hysteresis of elastic modulus in granular Y-Ba-Cu-O and Bi-Sr-Ca-Cu-O. Solid State Communications, 75:495–498, 8 1990. Palmer. 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spelling	Giraldo Gallo, Paula LilianaCruz Castiblanco, Juan Pablo NicolásRincón, JuliánRoa, JairoFacultad de Ciencias2024-01-31T20:12:44Z2025-02-192023-12-122024-01-30https://hdl.handle.net/1992/73704instname:Universidad de los Andesreponame:Repositorio Institucional Sénecarepourl:https://repositorio.uniandes.edu.co/During this master's thesis, the set-up of resonant ultrasound spectroscopy (RUS) technique was developed at the Universidad de los Andes and a temperature-dependent experiment was carried out.Durante esta tesis de maestría se desarrollo el montaje de la técnica de espectroscopía de resonancia ultrasónica (RUS) en la Universidad de los Andes y se llevó a cabo un experimento en función de la temperatura.Transition metal chalcogenides are an example of quantum materials, which show, topological states, charge density wave (CDW) formation, and ferroic orders. Within this family, the transition metal tetracalcogenides, NbTe4 and TaTe4, have captured the interest of the scientific community for being candidates to present axionic states connecting different Weyl points on the fermi surface through CDW formation. This represents a possibility to study the relationship between topological states of matter and correlated electronic states such as CDW. Diffraction, scanning tunneling spectroscopy, angle resolved photoemission spectroscopy and transport measurements have revealed important information about the CDW formation in these compounds. For instance, resistivity and diffraction measurements as a function of temperature in these materials suggest possible phase transitions at certain temperatures, which, for the case of NbTe4, could be related to reconfigurations of the CDW order. However, bulk thermodynamic measurements that can give more insight into the nature of such transitions are still missing. In this thesis we present resonant ultrasound spectroscopy (RUS) measurements for NbTe4 and TaTe4 single crystals, in order to get thermodynamic information of the reported putative phase transitions at different temperatures, through the determination of the temperature dependence of the elastic constants. For NbTe4 we find that the resonance frequencies, directly related to the elastic constants, are highly hysteretical in the temperature range of 100K to 300K, which can be directly related to the presence and dynamics of the recently reported CDW domain walls (DWs). In contrast, TaTe4 does not show such hysteretical behavior. These results suggest that DWs in NbTe4 play a fundamental role in both, the electronic and elastic properties of NbTe4.Los calcogenuros de metales de transición son un ejemplo de materiales cuánticos que muestran estados topológicos, formación de onda de densidad de carga (CDW) y orden ferroíco. Dentro de esta familia, los tetracalcogenuros de metales de transición, NbTe4 y TaTe4, han capturado el interés de la comunidad científica por ser candidatos a presentar estados axiónicos que conectan diferentes puntos de Weyl en la superficie de Fermi a través de la formación de CDW. Esto representa una oportunidad para estudiar la relación entre los estados topológicos de la materia y los estados electrónicos correlacionados, como la CDW. Mediciones de difracción, microscopía de efecto tunel (STM), espectroscopía de fotoemisión angular resuelta en energía (ARPES) y las mediciones de transporte han revelado información importante sobre la formación de CDW en estos compuestos. Por ejemplo, las mediciones de resistividad y difracción en función de la temperatura en estos materiales sugieren posibles transiciones de fase a ciertas temperaturas, que, en el caso del NbTe4, podrían estar relacionadas con reconfiguraciones del orden CDW. Sin embargo, aún faltan mediciones termodinámicas que puedan proporcionar una mayor comprensión de la naturaleza de tales transiciones. En esta tesis, presentamos mediciones de espectroscopía de resonancia ultrasónica (RUS) para monocristales de NbTe4 y TaTe4, con el fin de obtener información termodinámica sobre las posibles transiciones de fase reportadas a diferentes temperaturas, a través de la determinación de la dependencia de la temperatura de las constantes elásticas con la temperatura. Para NbTe4 encontramos que las frecuencias de resonancia, directamente relacionadas con las constantes elásticas, muestran un comportamiento altamente histeretico en el rango de temperatura de 100K a 300K, lo que puede estar directamente relacionado con la presencia y dinámica de las paredes de dominio (DW) de la CDW recientemente reportadas en este material. En contraste, el TaTe4 no muestra tal comportamiento histérico. Estos resultados sugieren que las DW en NbTe4 desempeñan un papel fundamental tanto en las propiedades electrónicas como elásticas del NbTe4.Universidad de los Andes, Facultad de Ciencias, Departamento de físicaTesis Magíster en Ciencias - FísicaMaestríaQuantum MaterialsCharge density wavePhase transitions128 páginasapplication/pdfspaUniversidad de los AndesMaestría en Ciencias-FísicaFacultad de CienciasDepartamento de FísicaAttribution 4.0 Internationalhttp://creativecommons.org/licenses/by/4.0/info:eu-repo/semantics/embargoedAccesshttp://purl.org/coar/access_right/c_f1cfResonant ultrasound spectroscopy of transition metal tetrachalcogenidesEspectroscopía de resonancia ultrasónica de calcogenuros de metales de transiciónTrabajo de grado - Maestríainfo:eu-repo/semantics/masterThesisinfo:eu-repo/semantics/acceptedVersionhttp://purl.org/coar/resource_type/c_7a1fTexthttp://purl.org/redcol/resource_type/TPCharge density waveNbTe4TaTe4Phase transitionsResonant ultrasound spectroscopyThermal hysteresisOnda de densidad de cargaNbTe4TaTe4Transisiones de faseEspectroscopía de resonancia ultrasónicaHistéresis térmicaFísicaJ. 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Resonant ultrasound spectroscopy of transition metal tetrachalcogenides

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