CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol

Powdered layered double hydroxides (LDH) based on calcium-aluminum (Ca–Al), nickel-aluminum (Ni–Al), and zinc-aluminum (Zn–Al) were synthesized with the purpose to evaluate the removal of o-nitrophenol from synthetic effluents by adsorption. It was verified that Ca–Al, Ni–Al, and Zn–Al LDHs presente...

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Autores:
Marques, Bianca S.
Dalmagro, Keterli
Moreira, Kelly S.
Oliveira, Marcos L.S.
Jahn, Sergio L.
De Lima Burgo, Thiago A.
Dotto, Guilherme L.
Tipo de recurso:
http://purl.org/coar/resource_type/c_816b
Fecha de publicación:
2020
Institución:
Corporación Universidad de la Costa
Repositorio:
REDICUC - Repositorio CUC
Idioma:
eng
OAI Identifier:
oai:repositorio.cuc.edu.co:11323/6300
Acceso en línea:
https://hdl.handle.net/11323/6300
https://doi.org/10.1016/j.jallcom.2020.155628
https://repositorio.cuc.edu.co/
Palabra clave:
Adsorption
General order
Layered structure
Nitrophenol
Simulated effluent
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oai_identifier_str oai:repositorio.cuc.edu.co:11323/6300
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network_name_str REDICUC - Repositorio CUC
repository_id_str
dc.title.spa.fl_str_mv CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
title CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
spellingShingle CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
Adsorption
General order
Layered structure
Nitrophenol
Simulated effluent
title_short CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
title_full CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
title_fullStr CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
title_full_unstemmed CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
title_sort CaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenol
dc.creator.fl_str_mv Marques, Bianca S.
Dalmagro, Keterli
Moreira, Kelly S.
Oliveira, Marcos L.S.
Jahn, Sergio L.
De Lima Burgo, Thiago A.
Dotto, Guilherme L.
dc.contributor.author.spa.fl_str_mv Marques, Bianca S.
Dalmagro, Keterli
Moreira, Kelly S.
Oliveira, Marcos L.S.
Jahn, Sergio L.
De Lima Burgo, Thiago A.
Dotto, Guilherme L.
dc.subject.spa.fl_str_mv Adsorption
General order
Layered structure
Nitrophenol
Simulated effluent
topic Adsorption
General order
Layered structure
Nitrophenol
Simulated effluent
description Powdered layered double hydroxides (LDH) based on calcium-aluminum (Ca–Al), nickel-aluminum (Ni–Al), and zinc-aluminum (Zn–Al) were synthesized with the purpose to evaluate the removal of o-nitrophenol from synthetic effluents by adsorption. It was verified that Ca–Al, Ni–Al, and Zn–Al LDHs presented a typical layered structure confirming the successful synthesis. o-nitrophenol adsorption on the LDH powders was favored at a pH of 5.0, being attained removal percentages from 70 to 90%, depending on the material. Kinetic experimental data obeyed the general order model, while, Sips represented the experimental equilibrium behavior of the three materials adequately. The maximum adsorption capacities were 135.1 mg g−1,122.1 mg g−1 and 130.3 mg g−1 for Ca–Al, Ni–Al, and Zn–Al LDHs, respectively. For simulated effluent, it was attained a removal of up to 60.3% using Ni–Al LDH. In a general way, the layered double hydroxides based on Ca–Al, Ni–Al, and Zn–Al exhibited an interesting potential as adsorbent materials for the treatment of simulated effluents containing o-nitrophenol. Ni–Al is preferred due to its better performance in the treatment of simulated effluents and higher regeneration potential.
publishDate 2020
dc.date.accessioned.none.fl_str_mv 2020-05-28T16:05:05Z
dc.date.available.none.fl_str_mv 2020-05-28T16:05:05Z
dc.date.issued.none.fl_str_mv 2020-05-13
dc.type.spa.fl_str_mv Pre-Publicación
dc.type.coar.spa.fl_str_mv http://purl.org/coar/resource_type/c_816b
dc.type.content.spa.fl_str_mv Text
dc.type.driver.spa.fl_str_mv info:eu-repo/semantics/preprint
dc.type.redcol.spa.fl_str_mv http://purl.org/redcol/resource_type/ARTOTR
dc.type.version.spa.fl_str_mv info:eu-repo/semantics/acceptedVersion
format http://purl.org/coar/resource_type/c_816b
status_str acceptedVersion
dc.identifier.uri.spa.fl_str_mv https://hdl.handle.net/11323/6300
dc.identifier.doi.spa.fl_str_mv https://doi.org/10.1016/j.jallcom.2020.155628
dc.identifier.instname.spa.fl_str_mv Corporación Universidad de la Costa
dc.identifier.reponame.spa.fl_str_mv REDICUC - Repositorio CUC
dc.identifier.repourl.spa.fl_str_mv https://repositorio.cuc.edu.co/
url https://hdl.handle.net/11323/6300
https://doi.org/10.1016/j.jallcom.2020.155628
https://repositorio.cuc.edu.co/
identifier_str_mv Corporación Universidad de la Costa
REDICUC - Repositorio CUC
dc.language.iso.none.fl_str_mv eng
language eng
dc.relation.references.spa.fl_str_mv [1] R. Arasteh, M. Masoumi, A.M. Rashidi, L. Moradi, V. Samimi, S. Mostafavi, Adsorption of 2-nitrophenol by multi-wall carbon nanotubes from aqueous solutions, Appl. Surf. Sci. 256 (2010) 4447e4455, https://doi.org/10.1016/ j.apsusc.2010.01.057.
[2] United States Environmental Protection Agency, Ambient water quality criteria for nitrophenols, in: In Canadian Cataloging in Publication Data 2, 1980. Issue October.
[3] S. Hamidouche, O. Bouras, F. Zermane, B. Cheknane, M. Houari, J. Debord, M. Harel, J.C. Bollinger, M. Baudu, Simultaneous sorption of 4-nitrophenol and 2-nitrophenol on a hybrid geocomposite based on surfactant-modified pillared-clay and activated carbon, Chem. Eng. J. 279 (2015) 964e972, https:// doi.org/10.1016/j.cej.2015.05.012.
[4] B. Kordi c, B. Jovi c, J. Trickovi c, M. Kovacevi c, Adsorption of selected nitrophenols on activated carbon in the presence of nicotinamide, J. Mol. Liq. 259 (2018) 7e15, https://doi.org/10.1016/j.molliq.2018.02.109.
[5] M.E. Mahmoud, G.M. Nabil, Nano zirconium silicate-coated manganese dioxide nanoparticles: microwave-assisted synthesis, process optimization, adsorption isotherm, kinetic study and thermodynamic parameters for removal of 4-nitrophenol, J. Mol. Liq. 240 (2017) 280e290, https://doi.org/ 10.1016/j.molliq.2017.05.075.
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[19] E.M. Seftel, R.G. Ciocarlan, B. Michielsen, V. Meynen, S. Mullens, P. Cool, Insights into phosphate adsorption behavior on structurally modified ZnAl layered double hydroxides, Appl. Clay Sci. 165 (2018) 234e246, https:// doi.org/10.1016/j.clay.2018.08.018.
[20] A. Elhalil, M. Farnane, A. Machrouhi, F.Z. Mahjoubi, R. Elmoubarki, H. Tounsadi, M. Abdennouri, N. Barka, Effects of molar ratio and calcination temperature on the adsorption performance of Zn/Al layered double hydroxide nanoparticles in the removal of pharmaceutical pollutants, J. Sci. Adv. Mater. Dev. 3 (2018) 188e195, https://doi.org/10.1016/j.jsamd.2018.03.005.
[21] E.H. Mourid, M. Lakraimi, L. Benaziz, E.H. Elkhattabi, A. Legrouri, Wastewater treatment test by removal of the sulfamethoxazole antibiotic by a calcined layered double hydroxide, Appl. Clay Sci. 168 (2018) 87e95, https://doi.org/ 10.1016/j.clay.2018.11.005
[22] T. Xiong, X. Yuan, X. Wang, Z. Wu, L. Jiang, L. Leng, K. Xi, X. Cao, G. Zeng, Highly efficient removal of diclofenac sodium from medical wastewater by Mg/Al layered double hydroxide-poly(m-phenylenediamine) composite, Chem. Eng. J. 366 (2019) 83e91, https://doi.org/10.1016/j.cej.2019.02.069.
[23] I.M. Ahmed, M.S. Gasser, Adsorption study of anionic reactive dye from aqueous solution to Mg-Fe-CO3 layered double hydroxide (LDH), Appl. Surf. Sci. 259 (2012) 650e656, https://doi.org/10.1016/j.apsusc.2012.07.092.
[24] F.P. De Sa, B.N. Cunha, L.M. Nunes, Effect of pH on the adsorption of Sunset Yellow FCF food dye into a layered double hydroxide (CaAl-LDH-NO3), Chem. Eng. J. 215e216 (2013) 122e127, https://doi.org/10.1016/j.cej.2012.11.024.
[25] F. Mohamed, M.R. Abukhadra, M. Shaban, M, Removal of safranin dye from water using polypyrrole nanofiber/Zn-Fe layered double hydroxide nanocomposite (Ppy NF/Zn-Fe LDH) of enhanced adsorption and photocatalytic properties, Sci. Total Environ. 640e641 (2018) 352e363, https://doi.org/ 10.1016/j.scitotenv.2018.05.316.
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[31] J.S. Piccin, T.R.S. Cadaval, L.A.A. Pinto, G.L. Dotto, Adsorption isotherms in liquid phase: experimental, modeling, and interpretations, in: A. BonillaPetriciolet, D.I. Mendoza-Castillo, H.E. Reynel-Avila (Eds.), Adsorption Pro- cesses for Water Treatment and Purification, Springer International Publishing, New York, 2017, pp. 19e51, https://doi.org/10.1007/978-3-319-58136-1_ 2.
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[39] M. Hu, X. Yan, X. Hu, R. Feng, M. Zhou, High-capacity adsorption of benzotriazole from aqueous solution by calcined Zn-Al layered double hydroxides, Colloid, Surf. A: Physicochem. Eng. Asp. 540 (2018) 207e214, https://doi.org/ 10.1016/j.colsurfa.2018.01.009.
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[42] A. Tor, Y. Cengeloglu, M.E. Aydin, M. Ersoz, Removal of phenol from aqueous phase by using neutralized red mud, J. Colloid Interface Sci. 300 (2006) 498e503, https://doi.org/10.1016/j.jcis.2006.04.054.
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spelling Marques, Bianca S.Dalmagro, KeterliMoreira, Kelly S.Oliveira, Marcos L.S.Jahn, Sergio L.De Lima Burgo, Thiago A.Dotto, Guilherme L.2020-05-28T16:05:05Z2020-05-28T16:05:05Z2020-05-13https://hdl.handle.net/11323/6300https://doi.org/10.1016/j.jallcom.2020.155628Corporación Universidad de la CostaREDICUC - Repositorio CUChttps://repositorio.cuc.edu.co/Powdered layered double hydroxides (LDH) based on calcium-aluminum (Ca–Al), nickel-aluminum (Ni–Al), and zinc-aluminum (Zn–Al) were synthesized with the purpose to evaluate the removal of o-nitrophenol from synthetic effluents by adsorption. It was verified that Ca–Al, Ni–Al, and Zn–Al LDHs presented a typical layered structure confirming the successful synthesis. o-nitrophenol adsorption on the LDH powders was favored at a pH of 5.0, being attained removal percentages from 70 to 90%, depending on the material. Kinetic experimental data obeyed the general order model, while, Sips represented the experimental equilibrium behavior of the three materials adequately. The maximum adsorption capacities were 135.1 mg g−1,122.1 mg g−1 and 130.3 mg g−1 for Ca–Al, Ni–Al, and Zn–Al LDHs, respectively. For simulated effluent, it was attained a removal of up to 60.3% using Ni–Al LDH. In a general way, the layered double hydroxides based on Ca–Al, Ni–Al, and Zn–Al exhibited an interesting potential as adsorbent materials for the treatment of simulated effluents containing o-nitrophenol. Ni–Al is preferred due to its better performance in the treatment of simulated effluents and higher regeneration potential.Marques, Bianca S.Dalmagro, KeterliMoreira, Kelly S.Oliveira, Marcos L.S.Jahn, Sergio L.De Lima Burgo, Thiago A.Dotto, Guilherme L.engCC0 1.0 Universalhttp://creativecommons.org/publicdomain/zero/1.0/info:eu-repo/semantics/openAccesshttp://purl.org/coar/access_right/c_abf2AdsorptionGeneral orderLayered structureNitrophenolSimulated effluentCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat synthetic effluents containing o-nitrophenolPre-Publicaciónhttp://purl.org/coar/resource_type/c_816bTextinfo:eu-repo/semantics/preprinthttp://purl.org/redcol/resource_type/ARTOTRinfo:eu-repo/semantics/acceptedVersion[1] R. Arasteh, M. Masoumi, A.M. Rashidi, L. Moradi, V. Samimi, S. Mostafavi, Adsorption of 2-nitrophenol by multi-wall carbon nanotubes from aqueous solutions, Appl. Surf. Sci. 256 (2010) 4447e4455, https://doi.org/10.1016/ j.apsusc.2010.01.057.[2] United States Environmental Protection Agency, Ambient water quality criteria for nitrophenols, in: In Canadian Cataloging in Publication Data 2, 1980. Issue October.[3] S. Hamidouche, O. Bouras, F. Zermane, B. Cheknane, M. Houari, J. Debord, M. Harel, J.C. Bollinger, M. Baudu, Simultaneous sorption of 4-nitrophenol and 2-nitrophenol on a hybrid geocomposite based on surfactant-modified pillared-clay and activated carbon, Chem. Eng. J. 279 (2015) 964e972, https:// doi.org/10.1016/j.cej.2015.05.012.[4] B. Kordi c, B. Jovi c, J. Trickovi c, M. Kovacevi c, Adsorption of selected nitrophenols on activated carbon in the presence of nicotinamide, J. Mol. Liq. 259 (2018) 7e15, https://doi.org/10.1016/j.molliq.2018.02.109.[5] M.E. Mahmoud, G.M. 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Kochany, Degradation of nitrobenzene and nitrophenols by means of advanced oxidation processes in a homogeneous phase: photolysis in the presence of hydrogen peroxide versus the Fenton reaction, Chemosphere 24 (1992) 1369e1380, https://doi.org/10.1016/0045-6535(92)90060-5.PublicationORIGINALCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.htmlCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.htmltext/html76290https://repositorio.cuc.edu.co/bitstreams/844718b8-710f-4701-a3da-9b8e767a8b27/downloade575731eb6aac221aaf904b32e6ddcbfMD51CC-LICENSElicense_rdflicense_rdfapplication/rdf+xml; charset=utf-8701https://repositorio.cuc.edu.co/bitstreams/bc7a50bd-11c8-48ec-91e9-8241a715ac1b/download42fd4ad1e89814f5e4a476b409eb708cMD52LICENSElicense.txtlicense.txttext/plain; charset=utf-81748https://repositorio.cuc.edu.co/bitstreams/77b1f8ad-bc9b-48e5-b4ca-eaa38fdf3f6f/download8a4605be74aa9ea9d79846c1fba20a33MD53TEXTCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.html.txtCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.html.txttext/plain3567https://repositorio.cuc.edu.co/bitstreams/7a746b5e-6196-43b2-8026-b9b763f3e61e/download751e6b39c164be93a6daf004187216bfMD54TEXTCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.html.txtCaeAl, NieAl and ZneAl LDH powders as efficient materials to treat.html.txttext/plain3567https://repositorio.cuc.edu.co/bitstreams/0929b42a-273e-4b8e-9d5e-a92ea4a9859d/download751e6b39c164be93a6daf004187216bfMD5411323/6300oai:repositorio.cuc.edu.co:11323/63002024-09-17 14:17:13.269http://creativecommons.org/publicdomain/zero/1.0/CC0 1.0 Universalopen.accesshttps://repositorio.cuc.edu.coRepositorio de la Universidad de la Costa CUCrepdigital@cuc.edu.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