Geochemical study of submicron particulate matter (PM1) in a metropolitan area

Air pollution has become a major problem in urban areas due to increasing industrialization and urbanization. In this study ambient concentrations of PM1 and metal concentrations as well as source contributions were identified and quantified by using Positive Matrix Factorization (PMF) in receptor m...

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Autores:
Schneider, Ismael
Teixeira, Elba C.
Dotto, Guilherme Luiz
Diana
Yang, Xue-cheng
Silva Oliveira, Luis Felipe
Tipo de recurso:
Article of journal
Fecha de publicación:
2020
Institución:
Corporación Universidad de la Costa
Repositorio:
REDICUC - Repositorio CUC
Idioma:
eng
OAI Identifier:
oai:repositorio.cuc.edu.co:11323/7651
Acceso en línea:
https://hdl.handle.net/11323/7651
https://doi.org/10.1016/j.gsf.2020.12.011
https://repositorio.cuc.edu.co/
Palabra clave:
PM1
Trace elements
Source apportionment
PMF
Back trajectory
Rights
openAccess
License
CC0 1.0 Universal
id RCUC2_af4ed17792a63a2af90b09f8d96bc59e
oai_identifier_str oai:repositorio.cuc.edu.co:11323/7651
network_acronym_str RCUC2
network_name_str REDICUC - Repositorio CUC
repository_id_str
dc.title.spa.fl_str_mv Geochemical study of submicron particulate matter (PM1) in a metropolitan area
title Geochemical study of submicron particulate matter (PM1) in a metropolitan area
spellingShingle Geochemical study of submicron particulate matter (PM1) in a metropolitan area
PM1
Trace elements
Source apportionment
PMF
Back trajectory
title_short Geochemical study of submicron particulate matter (PM1) in a metropolitan area
title_full Geochemical study of submicron particulate matter (PM1) in a metropolitan area
title_fullStr Geochemical study of submicron particulate matter (PM1) in a metropolitan area
title_full_unstemmed Geochemical study of submicron particulate matter (PM1) in a metropolitan area
title_sort Geochemical study of submicron particulate matter (PM1) in a metropolitan area
dc.creator.fl_str_mv Schneider, Ismael
Teixeira, Elba C.
Dotto, Guilherme Luiz
Diana
Yang, Xue-cheng
Silva Oliveira, Luis Felipe
dc.contributor.author.spa.fl_str_mv Schneider, Ismael
Teixeira, Elba C.
Dotto, Guilherme Luiz
Diana
Yang, Xue-cheng
Silva Oliveira, Luis Felipe
dc.subject.spa.fl_str_mv PM1
Trace elements
Source apportionment
PMF
Back trajectory
topic PM1
Trace elements
Source apportionment
PMF
Back trajectory
description Air pollution has become a major problem in urban areas due to increasing industrialization and urbanization. In this study ambient concentrations of PM1 and metal concentrations as well as source contributions were identified and quantified by using Positive Matrix Factorization (PMF) in receptor modeling in the Metropolitan Area of Porto Alegre, Brazil. The PM1 samples were collected on PTFE filters from December 2012 to December 2014 in two sampling sites. Major ion and trace element concentrations were assessed. The average concentrations were 12.8 and 15.2 μg/m3 for Canoas and Sapucaia do Sul sites, respectively. Major ion contributions of PM1 were secondary pollutants such as sulfate and nitrate. Trace elements, especially Cu, Pb, Zn, Cd, and Ni also made important contributions which are directly associated with anthropogenic contributions. Our results show significantly higher levels in winter than in summer. Most of the PM1 and the analyzed PM species and elements originated from anthropogenic sources, especially road traffic, combustion processes and industrial activities, which are grouped in 7 major contributing sources. A back-trajectory analysis showed that the long-range transport of pollutants was not relevant in relation to the contribution to PM1 and metal concentrations. This work highlights the importance of urban planning to reduce human health exposure to traffic and industrial emissions, combined with awareness-raising actions for citizens concerning the impact of indoor sources.
publishDate 2020
dc.date.issued.none.fl_str_mv 2020-12-30
dc.date.accessioned.none.fl_str_mv 2021-01-04T19:11:36Z
dc.date.available.none.fl_str_mv 2021-01-04T19:11:36Z
dc.type.spa.fl_str_mv Artículo de revista
dc.type.coar.fl_str_mv http://purl.org/coar/resource_type/c_2df8fbb1
dc.type.coar.spa.fl_str_mv http://purl.org/coar/resource_type/c_6501
dc.type.content.spa.fl_str_mv Text
dc.type.driver.spa.fl_str_mv info:eu-repo/semantics/article
dc.type.redcol.spa.fl_str_mv http://purl.org/redcol/resource_type/ART
dc.type.version.spa.fl_str_mv info:eu-repo/semantics/acceptedVersion
format http://purl.org/coar/resource_type/c_6501
status_str acceptedVersion
dc.identifier.issn.spa.fl_str_mv 1674-9871
dc.identifier.uri.spa.fl_str_mv https://hdl.handle.net/11323/7651
dc.identifier.doi.spa.fl_str_mv https://doi.org/10.1016/j.gsf.2020.12.011
dc.identifier.instname.spa.fl_str_mv Corporación Universidad de la Costa
dc.identifier.reponame.spa.fl_str_mv REDICUC - Repositorio CUC
dc.identifier.repourl.spa.fl_str_mv https://repositorio.cuc.edu.co/
identifier_str_mv 1674-9871
Corporación Universidad de la Costa
REDICUC - Repositorio CUC
url https://hdl.handle.net/11323/7651
https://doi.org/10.1016/j.gsf.2020.12.011
https://repositorio.cuc.edu.co/
dc.language.iso.none.fl_str_mv eng
language eng
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spelling Schneider, IsmaelTeixeira, Elba C.Dotto, Guilherme LuizDianaYang, Xue-chengSilva Oliveira, Luis Felipe2021-01-04T19:11:36Z2021-01-04T19:11:36Z2020-12-301674-9871https://hdl.handle.net/11323/7651https://doi.org/10.1016/j.gsf.2020.12.011Corporación Universidad de la CostaREDICUC - Repositorio CUChttps://repositorio.cuc.edu.co/Air pollution has become a major problem in urban areas due to increasing industrialization and urbanization. In this study ambient concentrations of PM1 and metal concentrations as well as source contributions were identified and quantified by using Positive Matrix Factorization (PMF) in receptor modeling in the Metropolitan Area of Porto Alegre, Brazil. The PM1 samples were collected on PTFE filters from December 2012 to December 2014 in two sampling sites. Major ion and trace element concentrations were assessed. The average concentrations were 12.8 and 15.2 μg/m3 for Canoas and Sapucaia do Sul sites, respectively. Major ion contributions of PM1 were secondary pollutants such as sulfate and nitrate. Trace elements, especially Cu, Pb, Zn, Cd, and Ni also made important contributions which are directly associated with anthropogenic contributions. Our results show significantly higher levels in winter than in summer. Most of the PM1 and the analyzed PM species and elements originated from anthropogenic sources, especially road traffic, combustion processes and industrial activities, which are grouped in 7 major contributing sources. A back-trajectory analysis showed that the long-range transport of pollutants was not relevant in relation to the contribution to PM1 and metal concentrations. This work highlights the importance of urban planning to reduce human health exposure to traffic and industrial emissions, combined with awareness-raising actions for citizens concerning the impact of indoor sources.Schneider, Ismael-will be generated-orcid-0000-0002-6217-4183-600Teixeira, Elba C.Dotto, Guilherme Luiz-will be generated-orcid-0000-0002-4413-8138-600DianaYang, Xue-cheng-will be generated-orcid-0000-0002-6860-7330-600Silva Oliveira, Luis Felipeapplication/pdfengCorporación Universidad de la CostaCC0 1.0 Universalhttp://creativecommons.org/publicdomain/zero/1.0/info:eu-repo/semantics/openAccesshttp://purl.org/coar/access_right/c_abf2Geoscience Frontiershttps://www.sciencedirect.com/science/article/pii/S167498712030270X#!PM1Trace elementsSource apportionmentPMFBack trajectoryGeochemical study of submicron particulate matter (PM1) in a metropolitan areaArtículo de revistahttp://purl.org/coar/resource_type/c_6501http://purl.org/coar/resource_type/c_2df8fbb1Textinfo:eu-repo/semantics/articlehttp://purl.org/redcol/resource_type/ARTinfo:eu-repo/semantics/acceptedVersionAgudelo-Castañeda, D.M., Teixeira, E.C., 2014. 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