Spatial distribution and chemical composition of road dust in two high-altitude Latin American cities

Road dust (RD) resuspension is one of the main sources of particulate matter in cities with adverse impacts on air quality, health, and climate. Studies on the variability of the deposited PM10 fraction of RD (RD10) have been limited in Latin America, whereby our understanding of the central factors...

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Autores:
Vanegas Gracia, Johan Sebastian
Trejos, Erika M.
Aristizábal, Beatriz H.
Pereira, Guilherme M.
Hernández, Julio M.
Herrera Murillo, Jorge
Ramírez, Omar
Amato, Fulvio
Silva Oliveira, Luis Felipe
Rojas, Nestor
Zafra Mejía, Carlos Alfonso
Pachon, Jorge E.
Tipo de recurso:
Article of journal
Fecha de publicación:
2021
Institución:
Corporación Universidad de la Costa
Repositorio:
REDICUC - Repositorio CUC
Idioma:
eng
OAI Identifier:
oai:repositorio.cuc.edu.co:11323/8996
Acceso en línea:
https://hdl.handle.net/11323/8996
https://doi.org/10.3390/atmos12091109
https://repositorio.cuc.edu.co/
Palabra clave:
PM10
Dust resuspension
Sediment load
Non-exhaust emissions
Chemical profile
Enrichment factors
Colombia
Rights
openAccess
License
CC0 1.0 Universal
Description
Summary:Road dust (RD) resuspension is one of the main sources of particulate matter in cities with adverse impacts on air quality, health, and climate. Studies on the variability of the deposited PM10 fraction of RD (RD10) have been limited in Latin America, whereby our understanding of the central factors that control this pollutant remains incomplete. In this study, forty-one RD10 samples were collected in two Andean cities (Bogotá and Manizales) and analyzed for ions, minerals, and trace elements. RD10 levels varied between 1.8–45.7 mg/m2, with an average of 11.8 mg/m2, in Bogotá and between 0.8–26.7 mg/m2, with an average of 5.7 mg/m2, in Manizales. Minerals were the most abundant species in both cities, with a fraction significantly larger in Manizales (38%) than Bogotá (9%). The difference could be explained mainly by the complex topography and the composition of soil derived from volcanic ash in Manizales. The volcanic activity was also associated with SO4−2 and Cl−. Enrichment factors and principal component analysis were conducted to explore potential factors associated to sources of RD10. Elements such as Cu, Pb, Cr, Ni, V, Sb, and Mo were mainly associated with exhaust and non-exhaust traffic emissions.