Quantum process tomography by 2D fluorescence spectroscopy

Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g.,...

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Fecha de publicación:: 2014

Institución:: Ministerio de Ciencia, Tecnología e Innovación

Repositorio:: Repositorio Minciencias

Idioma:: eng

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spelling	Colombia2019-03-17T21:35:16Z2019-03-17T21:35:16Z2014-10-07info:eu-repo/date/embargoEnd/2024-01-31http://repositorio.colciencias.gov.co/handle/11146/34071Contiene 38 referencias bibliográficas. Véase el documento adjunto10.1063/1.4919954Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed.Departamento Administrativo de Ciencia, Tecnología e Innovación [CO] Colciencias1115-569-34912nopdf10 páginasengBaños térmicos cuánticos: influencia de la no-gaussianidad estadística y no-localidad dinámica en la evolución temporal de sistemas cuánticos abiertos. La publicación completa está disponible en : <a href="http://repositorio.colciencias.gov.co/handle/11146/34053" target="blank">http://repositorio.colciencias.gov.co/handle/11146/34053</a>The Journal of Chemical Physics vol 142.212442 (10 pp). 2015Quantum process tomography by 2D fluorescence spectroscopyArtículo científicoinfo:eu-repo/semantics/articlehttp://purl.org/coar/version/c_970fb48d4fbd8a85http://purl.org/coar/resource_type/c_2df8fbb1Administradores de ciencia y tecnologíaInvestigadoresTermodinámicaModelos matemáticosMétodos de simulaciónDinámica de sistemasTeoría de campos (física)Propiedades termodinámicashttp://purl.org/coar/access_right/c_f1cfPachón, Leonardo AugustoMarcus, Andrew H.Aspuru-Guzik, AlánUniversidad de Antioquia, UdeAleonardo.pachon@fisica.udea.edu.co2013-02Programa Nacional de Ciencias BásicasComunidad científica colombiana0005-2013Artículos de investigaciónPublicationORIGINALQuantum process tomography by 2D fluorescence spectroscopy - copia.pdfQuantum process tomography by 2D fluorescence spectroscopy - copia.pdfArtículo The Journal of Chemical Physisapplication/pdf799187https://repositorio.minciencias.gov.co/bitstreams/3f1d9847-d1e6-4034-a673-b6c83f13cc67/download15ecb74088c94f5f66c02c08bacdbbbaMD51LICENSElicense.txtlicense.txttext/plain; charset=utf-81748https://repositorio.minciencias.gov.co/bitstreams/fd6f4621-3826-4c15-ac50-b43d60e8d4bc/download8a4605be74aa9ea9d79846c1fba20a33MD52TEXTQuantum process tomography by 2D fluorescence spectroscopy - copia.pdf.txtQuantum process tomography by 2D fluorescence spectroscopy - copia.pdf.txtExtracted texttext/plain10https://repositorio.minciencias.gov.co/bitstreams/340e2282-133f-404a-9556-5d07a8d651c7/download2c6eb67c8897d916ae47524b1a844d3fMD55THUMBNAILQuantum process tomography by 2D fluorescence spectroscopy - copia.pdf.jpgQuantum process tomography by 2D fluorescence spectroscopy - copia.pdf.jpgGenerated Thumbnailimage/jpeg18597https://repositorio.minciencias.gov.co/bitstreams/3bde52ee-ed41-4b2b-a924-3446765a26b4/downloadc3b121812cb99927d1bd11058a29ff37MD5620.500.14143/34071oai:repositorio.minciencias.gov.co:20.500.14143/340712023-11-29 17:28:16.502restrictedhttps://repositorio.minciencias.gov.coRepositorio Institucional de Mincienciascendoc@minciencias.gov.co
dc.title.es_CO.fl_str_mv	Quantum process tomography by 2D fluorescence spectroscopy
title	Quantum process tomography by 2D fluorescence spectroscopy
spellingShingle	Quantum process tomography by 2D fluorescence spectroscopy Termodinámica Modelos matemáticos Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
title_short	Quantum process tomography by 2D fluorescence spectroscopy
title_full	Quantum process tomography by 2D fluorescence spectroscopy
title_fullStr	Quantum process tomography by 2D fluorescence spectroscopy
title_full_unstemmed	Quantum process tomography by 2D fluorescence spectroscopy
title_sort	Quantum process tomography by 2D fluorescence spectroscopy
dc.subject.lemb.es_CO.fl_str_mv	Termodinámica Modelos matemáticos
topic	Termodinámica Modelos matemáticos Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
dc.subject.spines.es_CO.fl_str_mv	Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
description	Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed.
publishDate	2014
dc.date.issued.none.fl_str_mv	2014-10-07
dc.date.accessioned.none.fl_str_mv	2019-03-17T21:35:16Z
dc.date.available.none.fl_str_mv	2019-03-17T21:35:16Z
dc.date.embargoEnd.es_CO.fl_str_mv	info:eu-repo/date/embargoEnd/2024-01-31
dc.type.es_CO.fl_str_mv	Artículo científico
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dc.type.driver.es_CO.fl_str_mv	info:eu-repo/semantics/article
dc.identifier.uri.none.fl_str_mv	http://repositorio.colciencias.gov.co/handle/11146/34071
dc.identifier.bibliographicCitation.es_CO.fl_str_mv	Contiene 38 referencias bibliográficas. Véase el documento adjunto
dc.identifier.doi.none.fl_str_mv	10.1063/1.4919954
url	http://repositorio.colciencias.gov.co/handle/11146/34071
identifier_str_mv	Contiene 38 referencias bibliográficas. Véase el documento adjunto 10.1063/1.4919954
dc.language.iso.es_CO.fl_str_mv	eng
language	eng
dc.relation.ispartof.es_CO.fl_str_mv	Baños térmicos cuánticos: influencia de la no-gaussianidad estadística y no-localidad dinámica en la evolución temporal de sistemas cuánticos abiertos. La publicación completa está disponible en : <a href="http://repositorio.colciencias.gov.co/handle/11146/34053" target="blank">http://repositorio.colciencias.gov.co/handle/11146/34053</a>
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dc.format.es_CO.fl_str_mv	pdf
dc.format.extent.es_CO.fl_str_mv	10 páginas
dc.coverage.spatial.es_CO.fl_str_mv	Colombia
dc.source.es_CO.fl_str_mv	The Journal of Chemical Physics vol 142.212442 (10 pp). 2015
institution	Ministerio de Ciencia, Tecnología e Innovación
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Quantum process tomography by 2D fluorescence spectroscopy

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