Quantum process tomography by 2D fluorescence spectroscopy
Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g.,...
- Autores:
- Tipo de recurso:
- Fecha de publicación:
- 2014
- Institución:
- Ministerio de Ciencia, Tecnología e Innovación
- Repositorio:
- Repositorio Minciencias
- Idioma:
- eng
- OAI Identifier:
- oai:repositorio.minciencias.gov.co:20.500.14143/34071
- Acceso en línea:
- http://repositorio.colciencias.gov.co/handle/11146/34071
- Palabra clave:
- Termodinámica
Modelos matemáticos
Métodos de simulación
Dinámica de sistemas
Teoría de campos (física)
Propiedades termodinámicas
- Rights
- License
- http://purl.org/coar/access_right/c_f1cf
| Summary: | Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed. |
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