Quantum process tomography by 2D fluorescence spectroscopy

Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g.,...

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Fecha de publicación:: 2014

Institución:: Ministerio de Ciencia Tecnología e Innovación

Repositorio:: Repositorio Institucional de Minciencias

Idioma:: eng

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spelling	Quantum process tomography by 2D fluorescence spectroscopyTermodinámicaModelos matemáticosMétodos de simulaciónDinámica de sistemasTeoría de campos (física)Propiedades termodinámicasReconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed.Departamento Administrativo de Ciencia, Tecnología e Innovación [CO] Colciencias1115-569-34912no2019-03-17T21:35:16Z2019-03-17T21:35:16Z2014-10-07info:eu-repo/date/embargoEnd/2024-01-31Artículo científicoinfo:eu-repo/semantics/articlehttp://purl.org/coar/version/c_970fb48d4fbd8a85http://purl.org/coar/resource_type/c_2df8fbb1pdf10 páginasapplication/pdfhttp://repositorio.colciencias.gov.co/handle/11146/34071Contiene 38 referencias bibliográficas. Véase el documento adjunto10.1063/1.4919954The Journal of Chemical Physics vol 142.212442 (10 pp). 2015engBaños térmicos cuánticos: influencia de la no-gaussianidad estadística y no-localidad dinámica en la evolución temporal de sistemas cuánticos abiertos. La publicación completa está disponible en : <a href="http://repositorio.colciencias.gov.co/handle/11146/34053" target="blank">http://repositorio.colciencias.gov.co/handle/11146/34053</a>Colombiahttp://purl.org/coar/access_right/c_f1cfPachón, Leonardo AugustoMarcus, Andrew H.Aspuru-Guzik, Alánoai:repositorio.minciencias.gov.co:20.500.14143/340712023-11-29T17:28:16Z
dc.title.none.fl_str_mv	Quantum process tomography by 2D fluorescence spectroscopy
title	Quantum process tomography by 2D fluorescence spectroscopy
spellingShingle	Quantum process tomography by 2D fluorescence spectroscopy Termodinámica Modelos matemáticos Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
title_short	Quantum process tomography by 2D fluorescence spectroscopy
title_full	Quantum process tomography by 2D fluorescence spectroscopy
title_fullStr	Quantum process tomography by 2D fluorescence spectroscopy
title_full_unstemmed	Quantum process tomography by 2D fluorescence spectroscopy
title_sort	Quantum process tomography by 2D fluorescence spectroscopy
dc.subject.none.fl_str_mv	Termodinámica Modelos matemáticos Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
topic	Termodinámica Modelos matemáticos Métodos de simulación Dinámica de sistemas Teoría de campos (física) Propiedades termodinámicas
description	Reconstruction of the dynamics (quantum process tomography) of the single-exciton manifold in energy transfer systems is proposed here on the basis of two-dimensional fluorescence spectroscopy (2D-FS) with phase-modulation. The quantum-process-tomography protocol introduced here benefits from, e.g., the sensitivity enhancement ascribed to 2D-FS. Although the isotropically averaged spectroscopic signals depend on the quantum yield parameter r of the doubly excited-exciton manifold, it is shown that the reconstruction of the dynamics is insensitive to this parameter. Applications 2015 AIP to foundational and applied problems, as well as further extensions, are discussed.
publishDate	2014
dc.date.none.fl_str_mv	2014-10-07 2019-03-17T21:35:16Z 2019-03-17T21:35:16Z info:eu-repo/date/embargoEnd/2024-01-31
dc.type.none.fl_str_mv	Artículo científico info:eu-repo/semantics/article
dc.type.coarversion.fl_str_mv	http://purl.org/coar/version/c_970fb48d4fbd8a85
dc.type.coar.fl_str_mv	http://purl.org/coar/resource_type/c_2df8fbb1
dc.identifier.none.fl_str_mv	http://repositorio.colciencias.gov.co/handle/11146/34071 Contiene 38 referencias bibliográficas. Véase el documento adjunto 10.1063/1.4919954
url	http://repositorio.colciencias.gov.co/handle/11146/34071
identifier_str_mv	Contiene 38 referencias bibliográficas. Véase el documento adjunto 10.1063/1.4919954
dc.language.none.fl_str_mv	eng
language	eng
dc.relation.none.fl_str_mv	Baños térmicos cuánticos: influencia de la no-gaussianidad estadística y no-localidad dinámica en la evolución temporal de sistemas cuánticos abiertos. La publicación completa está disponible en : <a href="http://repositorio.colciencias.gov.co/handle/11146/34053" target="blank">http://repositorio.colciencias.gov.co/handle/11146/34053</a>
dc.rights.coar.fl_str_mv	http://purl.org/coar/access_right/c_f1cf
rights_invalid_str_mv	http://purl.org/coar/access_right/c_f1cf
dc.format.none.fl_str_mv	pdf 10 páginas application/pdf
dc.coverage.none.fl_str_mv	Colombia
dc.source.none.fl_str_mv	The Journal of Chemical Physics vol 142.212442 (10 pp). 2015
institution	Ministerio de Ciencia Tecnología e Innovación
repository.name.fl_str_mv
repository.mail.fl_str_mv
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Quantum process tomography by 2D fluorescence spectroscopy

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